Solvation vs. surface charge transfer: an interfacial chemistry game drives cation motion
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Electrolyte structure and ion solvation dynamics determine ionic conductivities, and ion (de)solvation processes dominate interfacial chemistry and electrodeposition barriers. We elucidate electrolyte effects facilitating or impeding Li+ diffusion and deposition, and evaluate structural and energetic changes during the solvation complex pathway from the bulk to the anode surface.
author list (cited authors)
Angarita-Gomez, S., & Balbuena, P. B.