Using clathrate hydrates for gas storage and gas-mixture separations: experimental and computational studies at multiple length scales Academic Article uri icon

abstract

  • © 2018, © 2018 Informa UK Limited, trading as Taylor & Francis Group. Clathrate hydrates have characteristic properties that render them attractive for a number of industrial applications. Of particular interest are the following two cases: (i) the incorporation of large amounts of gas molecules into the solid structure has resulted in considering hydrates as possible material for the storage/transportation of energy or environmental gases, and (ii) the selective incorporation of guest molecules into the solid structure has resulted in considering hydrates for gas-mixture separations. For the proper design of such industrial applications, it is essential to know accurately a number of thermodynamic, structural and transport properties. Such properties can either be measured experimentally or calculated at different scales that span the molecular scale-up to the continuum scale. By using clathrate hydrates as a particular case study, we demonstrate that performing studies at multiple length scales can be utilised in order to obtain properties that are essential to process design.

author list (cited authors)

  • Tsimpanogiannis, I. N., Costandy, J., Kastanidis, P., Meragawi, S. E., Michalis, V. K., Papadimitriou, N. I., ... Economou, I. G.

citation count

  • 5

publication date

  • August 2018