Electronic-resonance-enhanced coherent anti-Stokes Raman spectroscopy of nitric oxide
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A report on the dual-pump, electronic-resonance-enhanced coherent anti-Stokes Raman spectroscopy (CARS) technique was presented. The use of the dual-pump ERE CARS technique allows to separate clearly the process by which the Raman coherence is probed with a second pump beam. A significant resonant enhancement of nitric oxide CARS signal was observed and good agreement between calculated and experimental spectra was obtained.