Femtosecond multicolor pump-probe investigation of ultrafast electron transfer of (NH3)5RuIII NCRuII(CN)5- in solution
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abstract
Ultrafast measurements on (NH3)sRuIIINCRuII (CN)5- in solution reveal an ultrafast spectral component due to vibrationally unrelaxed stimulated emission, allowing for new insights on the interplay of solvent and solute degrees of freedom in an electron transfer reaction.