Transient structures of crystals and liquids: An x-ray diffraction and EXAFS study
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CBr 4 in solution was excited with 266nm picosecond pulses and the spectra and kinetics of the excited states, intermediate and final products were recorded. A long lived CBr 4 dissociation transient characterized by a broad absorption band with a maximum at 480 nm was found to be a solvent stabilized ion pair, (CBr +, // Br -) solv. EXAFS experiments reveal the structure of CBr 4 and the final dissociation products in solution. Time resolved EXAFS studies are performed to detect and determine the structure of the dissociation intermediates as a function of time, with a resolution of a few picoseconds and 0.02 A. Transient lattice structures have been observed in metalic nano-crystals after been heated with pulsed laser excitation. The distortion of the lattice of Au (111) 150 nm thick film as a function of time after excitation has been measured.
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26th International Congress on High-Speed Photography and Photonics