ADDITION OF ACRYLONITRILE TO ANIONIC TRANSITION-METAL HYDRIDES - AN IONIC MODEL FOR HOMOGENEOUS OLEFIN PROCESSES
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abstract
The anionic transition metal hydrides, HM(CO)4L- (M = Cr, W; L = CO, P(OMe)3) reacted with acrylonitrile and other activated olefins to yield thermally stable addition products, CH3CH(X)M(CO)4L-. Kinetic data and electronic substituent effects indicated an associative hydride transfer mechanism. 1981.